This simulation calculates the measured contact angle for a rough, heterogeneous surface using the Wenzel and Cassie laws. The contact surface is a mixture of materials A and B. Change the fraction of component A and the surface contact angles of each material (θA and θB) with sliders. Another slider changes the surface roughness; for a completely smooth surface, the surface roughness ratio used in the Wenzel equation is 1. The measured contact angle (θW) is calculated and displayed above the water droplet graphic; arrows on this plot show where θW is measured. Surfaces with water contact angles > 90° have low wettability and are considered hydrophobic, whereas < 90° means the surface has high wettability and is considered hydrophilic. When θW = 0°, complete wetting occurs.

The Cassie model is used to determine the apparent contact angle for a heterogeneous surface θC:

cos θC = fA cos θA + fB cos θB,

where fA and fB are the fractions of components A and B on the surface, and fB = 1 − fA; θA and θB are the flat contact angles for A and B.

The Wenzel apparent (or measured) contact angle θW and roughness ratio r is

cos θW = r cos θC,

where r is the actual area divided by the apparent area; for a completely smooth surface, r = 1, while for a rough surface, r > 1.

The droplet represents a spherical cap; its volume V (μL) based on the volume of a sphere of radius R is

V = (π/3) R3 (2 − 3 cos θW + cos3θW).

Solving for R (mm) and eliminating extraneous solutions gives

R = 31/3 V1/3 ⁄ (2π − 3π cos θW + π cos3θW)1/3.

The measured droplet height h (mm) is

h = RR sin(π/2 − θW).

Complete wetting occurs when θW = 0°, and no wetting occurs when θW = 180°.

Reference
[1] Wikipedia. "Wetting." (Oct 26, 2015) en.wikipedia.org/wiki/Wetting.

This simulation was created in the Department of Chemical and Biological Engineering at University of Colorado Boulder for LearnChemE.com by John L. Falconer using Claude AI. It is a JavaScript/HTML5 implementation of a Mathematica simulation by Rachael L. Baumann. It was prepared with financial support from the National Science Foundation (DUE 2336987 and 2336988) in collaboration with Washington State University. Address any questions or comments to LearnChemE@gmail.com.
surface contact angles (degrees):